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Figure 1.

Cartoon of model interactions.

The transmembrane death receptor Fas natively adopts a closed conformation, but can open to allow the binding of FADD, an adaptor molecule that facilitates apoptotic signal transduction. Open Fas can self-stabilize via stem helix and globular interactions, which is enhanced by receptor clustering through association with the ligand FasL.

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Figure 2.

Schematic of cluster-stabilization reactions.

Examples of ligand-independent cluster-stabilization reactions involving unstable () and stable () open receptors of molecularities two (A), three (B), and four (C). Higher-order reactions follow the same pattern. Ligand-dependent reactions are identical except that FasL () must be added to each reacting state.

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Figure 3.

Steady-state activation curves.

The steady-state active Fas concentration shows bistability and hysteresis as a function of the FasL concentration (stable, solid lines; unstable, dashed lines). At low receptor concentrations , the bistability is reversible, but irreversibility emerges for sufficiently high, representing a committed cell death decision. All parameters set at baseline values unless otherwise noted.

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Figure 4.

Steady-state activation surface.

The steady-state surface for the active Fas concentration as a function of the FasL and total Fas concentrations and , respectively, is folded, indicating the existence of singularities, across which the system's steady-state behavior switches between monostability and bistability (stable, blue; unstable, red). All parameters set at baseline values unless otherwise noted.

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Figure 5.

Steady state diagram.

Steady state diagram identifying the regions of parameter space supporting monostability (colored) or bistability (gray) as a function of the FasL and total Fas concentrations and , respectively. The monostable region is colored as a heat map corresponding to the steady-state active Fas concentration . Irreversible bistability is indicated by the extension of the bistable region to the axis .

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Figure 6.

Bistability thresholds.

The activation (red) and deactivation (blue) thresholds characterizing the bistable regime (green) are defined as the concentrations of FasL at which the steady-state active Fas concentration (black) switches discontinuously from one branch to the other (stable, solid line; unstable, dashed line).

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Figure 7.

Sensitivity analysis of bistability thresholds.

The robustness of the bistability thresholds is investigated by measuring the effects of perturbating the model parameters about baseline values. For each threshold-parameter pair, a normalized sensitivity is computed by linear regression. Top, sensitivities for the FasL thresholds ; bottom, sensitivities for the corresponding Fas thresholds at FasL concentrations , respectively.

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Figure 8.

Robustness of bistability.

The fraction of parameter sets that exhibit bistability as a function of the sampling variability follows the exponential form , where is the asymptotic bistable fraction. The fitted value of suggests that this robustness remains substantial even as .

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Figure 9.

Cell-level cluster integration.

The apoptotic signals of all Fas clusters are integrated to produce a normalized cell activation . The resulting hysteresis curve on as a function of the FasL concentration is graded due to the heterogeneity of the bistability thresholds across the clusters (top). Despite this variability, a strong linear dependence persists between (bottom; the valid region is shown in green).

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Figure 10.

Model discrimination using hyperactive mutants.

The wildtype response curve, giving the steady-state active wildtype Fas fraction as a function of the FasL concentration (stable, solid lines; unstable, dashed lines), of the cluster model varies with the mutant population fraction , reflecting receptor interactions absent in the crosslinking model. The total receptor concentration is fixed at . All parameters set at baseline values unless otherwise noted.

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Figure 11.

Model discrimination using steady-state invariants.

Steady-state invariants are fit to synthetic data generated from each model. For each model-data pair, the invariant error is minimized over the model parameter space. The results suggest that invariant minimization can correctly identify the model from the data.

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