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Table 1.

Illite water saturation under different hydration degree.

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Table 1 Expand

Fig 1.

Construction process of illite model.

(a) Illite original cell model; (b) Illite cell model after ion replacement; (c) Illite supercell model.

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Fig 1 Expand

Fig 2.

Molecular dynamics simulation process.

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Fig 2 Expand

Fig 3.

Temperature relaxation diagram under molecular dynamics; (a) The relaxation process under NVT; (b) Relaxation process under NPT.

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Fig 3 Expand

Fig 4.

Illite crystal structure parameters under different hydration degree.

(a) Lattice length parameter; (b) Density and volume parameters.

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Fig 4 Expand

Fig 5.

Evolution law of illite basic layer spacing in different environments.

(a) The evolution of interlayer spacing of hydrated illite at 25 °C; (b) The evolution of interlayer spacing of hydrated illite at 0.101 MPa; (c) The effect of pressure on interlayer spacing; (d) The effect of temperature on interlayer spacing.

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Fig 5 Expand

Fig 6.

Radial distribution function of hydrated illite with water saturation of 25.39% at 25 °C.

(a) Radial distribution function of potassium ions and oxygen atoms in water; (b) Radial distribution function of potassium ion and hydrogen atom in water.

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Fig 6 Expand

Fig 7.

Radial distribution function of hydrated illite with water saturation of 25.39% at 0.101 MPa.

(a) Radial distribution function of potassium ions and oxygen atoms in water; (b) Radial distribution function of potassium ion and hydrogen atom in water.

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Fig 7 Expand

Fig 8.

Radial distribution function of hydrated illite with different water saturation at 25 °C and 0.101 MPa.

(a) Radial distribution function of potassium ions and oxygen atoms in water; (b) Radial distribution function of potassium ion and hydrogen atom in water.

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Fig 8 Expand

Fig 9.

K + hydration parameters of illite interlayer.

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Fig 9 Expand

Fig 10.

Mean square displacement of water molecules between illite layers.

(a) Mean square displacement of water molecules under pressure; (b) Mean square displacement of water molecules under temperature; (c) Mean square displacement of water molecules under different water saturations.

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Fig 10 Expand

Fig 11.

Mechanism of temperature effect on mechanical properties.

(a) bulk modulus; (b) Shear modulus; (c) Young ‘s modulus; (d) Poisson ‘s ratio.

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Fig 11 Expand

Fig 12.

Mechanism of pressure effect on mechanical properties.

(a) bulk modulus; (b) Shear modulus; (c) Young ‘s modulus; (d) Poisson ‘s ratio.

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Fig 12 Expand

Fig 13.

Mechanism of water saturation on mechanical properties.

(a) bulk modulus; (b) Shear modulus; (c) Young ‘s modulus; (d) Poisson ‘s ratio.

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Fig 13 Expand

Fig 14.

Evolution law of mechanical heterogeneity of hydrated illite.

(a) Coefficient of variation of bulk modulus; (b) Coefficient of variation of shear modulus; (c) Young ‘s modulus coefficient of variation; (d) Coefficient of variation of Poisson ‘s ratio.

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Fig 14 Expand