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Fig 1.

Identification of structural templates and domain boundaries of Taq DNA polymerase.

The full-length Taq DNA polymerase sequence (green bar, residues 1-832) was analyzed using the MODELLER program. The most homologous structural templates are aligned from top to bottom, with their corresponding PDB IDs shown in red boxes. A clear discontinuity between residues 290 and 293 (indicating by two vertical black lines) marks the structural boundary separating the N-terminal exonuclease domain (residues 1-290) and the C-terminal polymerase domain (residues 293-832).

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Fig 2.

Purification analysis of Taq-P and Taq-N proteins.

The purities of Taq-P and Taq-N were analyzed by reducing 4-12% gradient SDS-PAGE, and both proteins were used as antigens for mouse immunization. Lane M: Molecular weight marker; Taq-P protein: ~ 60 kDa; Taq-N protein: ~ 33 kDa.

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Fig 3.

Purification analysis of monoclonal antibodies.

Antibodies were analyzed by reducing 4-12% gradient SDS-PAGE. Lane M: Molecular weight marker; Lane 1: IgG Taq-N-A7; Lane 2: IgG Taq-P-B3; Lane 3: IgG Taq-P-D4. The observed bands at approximately 55 kDa and 25 kDa correspond to the immunoglobulin heavy chain (HC) and light chain (LC), respectively.

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Fig 4.

Determination of monoclonal antibody titers by indirect ELISA.

(A) Titers against full-length Taq DNA polymerase. (B) Titers against the Taq-N protein fragment. (C) Titers against the Taq-P protein fragment. PBST was used as the negative control. The results demonstrate that IgG Taq-N-A7 specifically binds to the Taq-N fragment, while IgG Taq-P-B3 and IgG Taq-P-D4 are specific for the Taq-P fragment.

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Fig 5.

Evaluation of Taq polymerase blocking by monoclonal antibodies using qPCR.

(A-C) PCR amplification curves obtained with Taq polymerase pre-incubated with different masses (0.25, 0.5, and 1 μg) of (A) IgG Taq-P-B3, (B) IgG Taq-N-A7, and (C) IgG Taq-P-D4. The reactions used a hairpin oligonucleotide (TZ) as template. Commercial hot-start Taq polymerase and unblocked Taq polymerase were used as positive and negative controls, respectively. The flat baseline during the initial 20 cycles at 70°C in (A) indicates complete enzyme inhibition by IgG Taq-P-B3 at 0.5 and 1 μg, while its activity was restored upon heating to 95°C. In contrast, IgG Taq-N-A7 and IgG Taq-P-D4 showed no significant blocking effect at any concentration tested.

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Fig 6.

Specificity analysis of hot-start PCR by qPCR.

(A, B) Melting curves (A1, B1) and amplification curves (A2, B2) from qPCR assays using IgG Taq-P-B3-blocked Taq polymerase (HS Taq) at template concentrations of 0.1 ng/μL (A) and 1 ng/μL (B). A commercial hot-start Taq enzyme served as the control.

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Fig 7.

Performance validation in a fungal detection assay.

Amplification curve analysis for the detection of Lichtheimia corymbifera using (A) the experimental HS Taq (blocked by IgG Taq-P-B3) and (B) a commercial hot-start Taq enzyme (control). The Ct values and curve profiles between the experimental and control groups are nearly identical.

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Table 1.

Comparison of Ct values and reproducibility between the experimental and commercial hot-start Taq polymerases in the Lichtheimia corymbifera detection assay.

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Table 1 Expand

Fig 8.

Comparative sensitivity analysis of hot-start Taq enzymes at low template concentrations.

Detection rates for Lichtheimia corymbifera at template concentrations of 300 copies/mL (A, B) and 75 copies/mL (C, D) are shown. (A, C) Results using a commercial hot-start Taq enzyme. (B, D) Results using the experimental HS Taq prepared with IgG Taq-P-B3. Each panel shows the number of positive detections out of 16 replicate reactions (e.g., 12/16).

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Fig 9.

Performance validation in a multiplex respiratory virus detection system.

(A) Melting curves for H1N1 detection (Peak 1) and (B) for simultaneous detection of PIV-1 (Peak 1) and PIV-3 (Peak 2). The experimental group (A1, B1) used HS Taq prepared with IgG Taq-P-B3, while the control group (A2, B2) used a commercial hot-start Taq enzyme. The absence of non-specific peaks and the concordance in Tm values between experimental and control groups.

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