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Fig 1.

Effect of different mass ratios on the adsorption properties of phosphate (P concentration = 100 mg/L, pH = 7, material dosage = 1 g/L, T = 25 ± 2.5 °C).

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Fig 1 Expand

Fig 2.

(a) The SEM image of SBC, (b-c) The SEM image of ESBC-1, (d-f) The EDS elemental diagram of ESBC-1 and (i) the Mapping spectrum of ESBC-1.

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Fig 2 Expand

Table 1.

Comparison of SBET, Total pore volume, and APD for SBC, ESBC-1, and ESBC-1-P (after phosphate adsorption).

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Table 1 Expand

Fig 3.

(a) Adsorption and desorption curve, (b-d) FTIR spectra, XRD patterns, and XPS spectra of SBC and ESBC-1.

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Fig 3 Expand

Table 2.

The elemental composition (atomic %) measured by XPS.

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Table 2 Expand

Table 3.

Parameters of adsorption isotherm models for phosphate adsorption by ESBC-1 and SBC at 298 K.

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Table 3 Expand

Fig 4.

(a-b) Adsorption isotherm models fitting for phosphate adsorption by SBC and ESBC-1, (c) Kinetic models fitting for phosphate adsorption by SBC, (d) Kinetic models fitting for phosphate adsorption by ESBC-1 (P concentration = 100 mg/L, pH = 7, material dosage = 1 g/L, T = 25 ± 2.5 °C).

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Fig 4 Expand

Table 4.

ESBC-1 and SBC adsorption kinetic parameters of phosphate.

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Table 4 Expand

Fig 5.

(a) Effect of dosage on phosphate adsorption, (b) Effect of initial pH on phosphate adsorption by ESBC-1, (c) Effect of coexisting ions on phosphate adsorption, (d) Phosphate adsorption performance of ESBC-1 and SBC in real biogas slurry (P concentration = 100 mg/L, initial pH = 7, material dosage = 1 g/L, T = 25 ± 2.5 °C unless specified differently).

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Fig 5 Expand

Fig 6.

SEM-EDS image of ESBC-1 after phosphate adsorption.

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Fig 6 Expand

Fig 7.

(a) FTIR spectra of ESBC-1 before and after phosphate adsorption, (b) XRD spectra of ESBC-1 before and after phosphate adsorption.

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Fig 7 Expand

Fig 8.

(a) XPS spectra of ESBC-1 before and after phosphate adsorption, (b) Ca 2p spectra of ESBC-1 before phosphate adsorption, (c) Ca 2p spectra of ESBC-1 after phosphate adsorption, (d) P 2p spectra of ESBC-1 after phosphate adsorption.

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Fig 8 Expand