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Fig 1.

Cr(VI) removal performance by M-Fe and M-Fe/Cu with different Fe/Cu mass ratio (the initial concentration of Cr(VI): 20 mg/L, pH

= 7, T = 25oC).

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Fig 1 Expand

Fig 2.

The XPS patterns of M-Fe/Cu-2: (a) Fe 2p and (b) Cu 2p.

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Fig 2 Expand

Fig 3.

The effect of initial pH on the removal of Cr(VI) (a); the kobs and the removal efficiency at 2 h (b) (the initial concentration was 20 mg/L Cr(VI), T

= 25oC).

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Fig 3 Expand

Fig 4.

The effect of initial Cr(VI) concentration for the Cr(VI) reduction: the removal efficiency at 2 h (a) and the kobs (b) (pH

= 7, T = 25oC).

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Fig 4 Expand

Fig 5.

Cr 2p XPS analysis of M-Fe/Cu-2 after reaction for different time: (a) 5 min, (b) 15 min, (c) 60 min, (d) 90 min, (e) 180min, (f) 360 min.

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Fig 5 Expand

Fig 6.

Fractions of Fe, Cu and Cr with different valence states in specific reaction time during the progress of Cr(VI) removal by M-Fe/Cu-2 according to the results of XPS spectra: (a) Fe, (b) Cu, (c) Cr.

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Fig 6 Expand

Fig 7.

Fe 2p XPS analysis of M-Fe/Cu-2 after reaction for different time: (a) 5 min, (b) 15 min, (c) 60 min, (d) 90 min, (e) 180min, (f) 360 min.

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Fig 7 Expand

Fig 8.

Cu 2p XPS analysis of M-Fe/Cu-2 after reaction for different time: (a) 5 min, (b) 15 min, (c) 60 min, (d) 90 min, (e) 180min, (f) 360 min.

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Fig 8 Expand

Fig 9.

Schematic diagram of Cr(VI) removal by M-Fe/Cu-2.

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Fig 9 Expand