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Fig 1.

Synthetic scheme of c(RGDfK)-SH.

To introduce thiol into c(RGDfK), SATA was conjugated to c(RGDfK). Subsequently, the sulfhydryl group was deprotected using hydroxylamine.

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Table 1.

Lipid composition of the liposomes.

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Table 1 Expand

Fig 2.

Particle size distribution curves of RGD-liposomes and NT-liposomes.

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Fig 3.

Inhibition of 125I-echistatin binding to αvβ3 integrin on PANC-1 cells by RGD-, RKG-, and NT-liposomes (n = 3).

The x-axis represents the concentration of the liposomal membrane lipid. The RGD-liposomes dose-dependently inhibited the binding of 125I-echistatin to PANC-1 cells in a dose-dependent manner. However, no inhibition was observed with RKG- or NT-liposomes.

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Fig 4.

Biodistribution of 111In-RGD-liposomes and 111In-NT-liposome in PANC-1 xenograft-bearing nude mice at 24 h post-injection (n = 3–4).

Results are expressed as the percentage of the ID/g tissue. The 111In-NT-liposome showed the highest accumulation in both tumor and blood. Among the 111In-RGD-liposomes, the 111In-H-RGD-liposome showed the lowest accumulation in these tissues. Accumulation in the spleen varied with the degree of RGD peptide modification on the liposomes.

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Fig 5.

Tumor-to-blood, -pancreas, and -muscle ratios of 111In-RGD-liposomes and 111In-NT-liposomes in PANC-1 xenograft-bearing nude mice at 24 h post-injection (n = 4).

Tumor to normal tissue ratios were calculated from the biodistribution data.

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Fig 5 Expand

Fig 6.

MR imaging (9.4 T) of PANC-1 xenograft-bearing scid mice.

(a) RARE T1 MR images after treatment with H-RGD-liposomes loaded with ferrioxamine B. Open arrowheads indicate enhanced areas. (b) RARE T1 MR images after treatment with RKG-liposomes loaded with ferrioxamine B. (c) Tumor-to-muscle signal (T/M) ratios for H-RGD- and RKG-liposomes loaded with ferrioxamine B (n = 3).

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