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Fig 1.

(A) Particle sizes and zeta potentials of FNP and PVA functionalized FNP (FNP/PVA) at different PVA concentrations of 1% (FNP/PVA 1), 3% (FNP/PVA 3), and 5% (FNP/PVA 5); (B) Particle sizes of CIP loaded FNP and FNP/PVA (n = 3); (C-F) SEM images of (C) FNP, (D) FNP/PVA, (E) CIP loaded FNP, and (F) CIP loaded FNP/PVA.

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Fig 1 Expand

Table 1.

Entrapment efficiency (EE%) of the CIP loaded FNP (FNP-CIP) and CIP loaded PVA functionalized FNP (FNP/PVA-CIP) (n = 3).

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Table 1 Expand

Fig 2.

(A-C) FT-IR spectra of silk fibroin (SF), FNP, and PVA functionalized FNP (FNP/PVA) at different PVA concentrations of 1% (FNP/PVA 1), 3% (FNP/PVA 3), and 5% (FNP/PVA 5); (A) the blank particles, (B) the CIP loaded particles formulated by the desolvation method, and (C) the CIP loaded particles formulated by the adsorption method; (D) DSC graphs and (E) XRD spectra of FNP, FNP/PVA, FNP-CIP, and FNP/PVA-CIP.

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Fig 2 Expand

Fig 3.

Adsorption process of CIP onto the FNP and PVA functionalized FNP (FNP/PVA) at different PVA concentrations; the particle isotherm models of (A) Langmuir and (B) Dubinin-Radushkevich; the kinetics models of (1) pseudo first-order and (2) pseudo second-order.

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Fig 3 Expand

Table 2.

Total number of CIP molecules and CIP charge moieties during the adsorption process.

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Table 2 Expand

Fig 4.

Summary of interactions between CIP and FNP during the adsorption process in water at pH 6.2.

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Fig 4 Expand

Fig 5.

Drug release patterns, in simulated gastrointestinal condition, of CIP from the FNP-CIP and PVA functionalized FNP (FNP/PVA-CIP), formulated using (A) the desolvation method and (B) the adsorption method (n = 3).

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Fig 5 Expand

Table 3.

MIC values of CIP loaded FNP (FNP-CIP) and PVA functionalized FNP (FNP/PVA-CIP) on Bacillus subtilis, Salmonella enterica, and Escherichia coli (n = 3).

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Table 3 Expand