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Table 1.

Physicochemical properties of biochars.

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Table 1 Expand

Table 2.

BET characteristics of biochars.

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Table 2 Expand

Fig 1.

Adsorption kinetic curves with different types of biochars.

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Fig 1 Expand

Table 3.

Kinetic model parameters for the fluorine adsorption using biochars.

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Table 3 Expand

Fig 2.

Fluorine kinetic adsorption curves using different soil samples.

(Note: a, swine manure biochar (350°C)-treated soil; b, swine manure biochar (500°C)-treated soil; c, swine manure biochar (650°C)-treated soil; d, straw biochar (500°C)-treated soil).

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Fig 2 Expand

Table 4.

Kinetic model parameters for the fluorine adsorption in biochar treated soils.

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Table 4 Expand

Fig 3.

Adsorption isotherms curves on biochars.

(Note: weight of biochar = 0.1 g, solution volume = 20 mL, pH = 7, 25°C).

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Fig 3 Expand

Table 5.

Adsorption isotherm parameters for the fluorine adsorption using biochars.

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Table 5 Expand

Table 6.

Comparison of fluorine adsorption capacities for PBC650 and RBC500 with for previously reported adsorbents.

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Table 6 Expand

Fig 4.

Adsorption isotherms curves in biochar treated soil samples.

(Note: weight of soil = 1.0 g, solution volume = 20 mL, pH = 7, 25°C).

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Fig 4 Expand

Table 7.

Adsorption isotherm parameters for the fluorine adsorption in biochar treated soils.

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Table 7 Expand

Table 8.

X2 statistics of two models.

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Table 8 Expand

Table 9.

Desorption isotherm parameters for the fluorine desorption in different soil samples.

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Table 9 Expand

Fig 5.

Adsorption curves using different biochars under different pH.

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Fig 5 Expand

Fig 6.

Soil adsorption curves under different pH.

(Note: a, PBC350-treated soil; b, PBC500-treated soil; c, PBC650-treated soil; d, RBC500-treated soil).

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Fig 6 Expand

Fig 7.

Effect of interfering ions at different concentrations on fluoride adsorption.

(Note: weight of biochar = 0.1 g, solution volume = 20 mL, CK is 50 mg/L of F-, interfering ions concentration = 50 mg/L、100 mg/L and 200 mg/L, pH = 7, 25°C).

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Fig 7 Expand

Fig 8.

Infrared spectra before and after biochar adsorption.

(Note: a, PBC350-treated soil; b, PBC500-treated soil; c, PBC650-treated soil; d, RBC500-treated soil).

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Fig 8 Expand

Fig 9.

SEM images of different types of biochars.

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