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Fig 1.

Example MS data of a of a strain of Salmonella enterica subsp. enterica serovar infantis.

(A) Linear MS data of bacterial cell lysate. (B) The identified protein sequence (hypothetical/YahO) after removal of its 21-residue signal peptide. An asterisk denotes a site of backbone cleavage with its corresponding b-type and/or y-type fragment ions. (C) MS/MS data of the protein ion at m/z 7666. Fragment ions are identified by m/z (theoretical value in parentheses) and their b- or y-type fragment ion designation. (D) The pre-processed and centroided MS/MS data of the protein ion at m/z 7666. Pre-processed and centroided MS/MS data is shown in Fig 1D.

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Fig 1 Expand

Fig 2.

Workflow for analysis of the selected bacterial proteins.

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Fig 2 Expand

Fig 3.

Distribution of D-, E-, and N-fragment signal scores.

(A) Histogram of D-, E-, and N- fragment scores. (B) Empirical cumulative distribution functions of D-, E-, and N-fragment scores.

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Fig 3 Expand

Table 1.

Multivariate regression analysis results.

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Table 1 Expand

Fig 4.

Distribution of D-, E-, and N- fragment signal scores with respect to significant explanatory variables.

(A-C) Empirical cumulative distribution functions (eCDF) of D-fragment signal scores. (D) eCDF of N-fragment signal scores. (E-I) eCDF of E-fragment signal scores. Shades of pink represent percentile of significant explanatory variable values.

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Fig 4 Expand

Fig 5.

Analysis of categorical explanatory variables.

(A) Box plot of fragment signal scores grouped by C-terminal residues adjacent to D. (B) Box plot of fragment signal scores grouped by C-terminal residues adjacent to E. (C) Box plot of fragment signal scores grouped by C-terminal residues adjacent to N. (D) Bar graph comparing the proline fragment signal scores whose adjacent N-terminal adjacent residue was D,E,N or non-D,E,N. (E) Box plot of fragment signal scores grouped by secondary structure of E-residues. Significant explanatory variables p<0.05, p<0.01, p<0.00001 is respectively marked by *,**, and ***** based on the Mann-Whitney U test. Bar graph is displayed as mean ± standard error.

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Fig 5 Expand

Table 2.

Kruskal-Wallis test of categorical explanatory variables.

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Table 2 Expand