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Table 1.

Characteristics of plasma pools.

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Fig 1.

Characterization of the EVs isolated by UC and AS.

(A) EVs quantification by NTA (particles/mL; mean ± SD; n = 3 independent reading for each condition). (B) Diameter of particles measured by NTA (mean ± SD; n = 3 independent reading for each condition). *, Student’s T-test, p< 0.05. (C) Western blot analysis of the EVs markers (HSP70 and CD9, CD63 and CD81 tetraspanins) and plasma contaminants (APOA1, APOB48/B100 and albumin) in UC- and AS-EVs.

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Fig 2.

Characterization of the surface epitopes of UC- and AS-EVs by using the MACSPlex kit.

Venn diagrams showing the overlap of the markers identified with the MACSPlex kit in UC-EVs_cit (A), UC-EVs_EDTA (B), AS-EVs_cit (C) and AS-EVs_EDTA (D). (E)Histograms showing the normalized MFI of the 19 markers shared by UC- and AS-EVs (mean ± SD). ***, Student’s T-test, p< 0.001. (F)PCA score plot for the markers detected by the MACPlex kit illustrating the relationship between the different EVs preparations. UC-EVs_cit = blue, UC-EVs_EDTA = light-blue, AS-EVs_cit = red, AS-EVs_EDTA = green. Circles represent the 95% confidence interval. (G) Heatmap of the unsupervised hierarchical clustering of surface epitopes investigated with the MACSPlex kit in UC- and AS-EVs. Autoscaling samples and Euclidean distance measure were applied.

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Fig 3.

Statistical analysis of the lipidomic data of the isolated EVs.

PCA (A) and PLS-DA (B) score plots for the lipids detected by untargeted lipidomic analysis displaying the separation between and UC- (blue and light-blue) and AS-EVs (red and green) and no separation between EVs_cit and EVs_EDTA, when purified with the same isolation method. Circles represent the 95% confidence interval. Volcano plot showing the lipid species that are statistically different (Student’s T-test, p< 0.05) between UC-EVs_cit and UC-EVs-EDTA (C) and between AS-EVs_cit and AS-EVs_EDTA (D). The X-axis represents the Log2-transformed FC and the Y-axis represents the log10-transformed p-value. In red the species that are significantly more expressed in citrate, in blue the species significantly more expressed in EDTA.

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Fig 4.

Analysis of the main lipid categories and classes regardless of the anticoagulant.

(A) Fold change (FC) of the main lipid categories in UC- versus AS-EVs. All the classes were statistically different, SL and GPL higher in UC-EVs while GL and FA and derivatives higher in AS-EVs. ***, Student’s T-test, p< 0.001. (B) FC and statistical analysis for each lipid class (UC- versus AS-EVs). **, Student’s T-test, p< 0.01; ***, Student’s T-test, p< 0.001.S3.

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Fig 5.

Characterization of the main lipid categories and classes regardless of the anticoagulant.

(A) Volcano plot showing the lipid species that are statistically different (fold change> 1.5; Student’s T-test, p< 0.05) between UC- and AS-EVs. The X-axis represents the Log2-transformed FC and the Y-axis represents the log10-transformed p-value. In red the species that are significantly more expressed in UC-EVs, in blue the species significantly more expressed in AS-EVs. (B) Heatmap of the unsupervised hierarchical clustering of the top 50 deregulated lipid species in order of p-value (UC-EVs versus AS-EVs) detected by untargeted lipidomic analysis in UC- and AS-EVs.

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