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Table 1.

Minimal inhibitory concentration (MIC) of IBP obtained for the tested actinobacterial strains.

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Table 1 Expand

Table 2.

Percentage of IBP (100 mg/L) remaining during biodegradation experiment after 7 days of incubation of the actinobacterial strains in the RS medium.

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Table 2 Expand

Fig 1.

Biodegradation rate of IBP (A), carbon dioxide release (B) and oxygen uptake (C) by R. cerastii IEGM 1278. 1 –dry weight (CDW) of rhodococcal biomass in the presence of IBP and n-hexadecane; 2 –dry weight of rhodococcal biomass in the presence of n-hexadecane. Cells were pre-grown in NB for 3 days. Biodegradation experiments were conducted in the RS medium supplemented with 0.1% n-hexadecane. The graph shows mean values ± SD of three experiments done in triplicate.

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Fig 1 Expand

Fig 2.

Biodegradation rate of IBP by R. cerastii IEGM 1278 in a laboratory bioreactor.

Biodegradation experiments were conducted in the RS medium supplemented with 0.1% n-hexadecane. The graph shows mean values ± SD of three experiments.

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Fig 2 Expand

Fig 3.

Biodegradation rate of IBP by native and pre-incubated R. cerastii IEGM 1278 cells.

1 –dry weight (CDW) of biomass in the presence of IBP and n-hexadecane; 2 –dry weight of biomass in the presence of n-hexadecane. Biodegradation experiments were conducted in the RS medium supplemented with 0.1% n-hexadecane. The graph gives mean values ± SD of three experiments done in triplicate.

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Fig 3 Expand

Fig 4.

Proposed scheme of IBP biotransformation by R. cerastii IEGM 1278.

1 –ibuprofen sodium salt; 2 –ibuprofen; 3–9-hydroxy ibuprofen; 4–6,9-dihydroxy ibuprofen; 5–6-hydroxy ibuprofen; 6 –decarboxylated derivative of 9-hydroxy ibuprofen; 7 –decarboxylated derivative of 6,9-dihydroxy ibuprofen; 8 –decarboxylated derivative of 6-hydroxy ibuprofen. The numbering of IBP atoms proposed by Preskar et al. is used [88].

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Fig 4 Expand

Table 3.

Experimental phytotoxicity of IBP and its biotransformation products.

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Table 3 Expand

Table 4.

Toxicity of IBP (1–2) and its biotransformation products (3–7) calculated using ECOSAR.

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Table 4 Expand

Table 5.

Soil sorption, bioconcentration and bioaccumulation of IBP and its transformation products calculated using EPI Suite.

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Table 5 Expand

Table 6.

Biodegradability of IBP and its biotransformation products calculated using EPI Suite.

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Table 6 Expand

Fig 5.

Cell aggregates of R. cerastii IEGM 1278.

A–culture flask; B–phase-contrast image, x 1,000. 1 –cords; 2 –bacterial cells. Cells were grown for 3 days in the RS medium supplemented with 0.1% n-hexadecane and 100 mg/L IBP.

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Fig 5 Expand

Fig 6.

CLSM (A) and AFM (B, C) images and profiles (D) of R. cerastii IEGM 1278. Cells were grown for 24 h in the RS medium supplemented with 0.1% n-hexadecane (I) and 100 mg/L IBP and 0.1% n-hexadecane (II). The scale bars on the CLSM images correspond to 5 μm.

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Fig 6 Expand

Fig 7.

CLSM (A) and AFM (B, C) images and profiles (D) of R. cerastii IEGM 1278. Cells were grown for 4 days in the RS medium supplemented with 0.1% n-hexadecane (I) and 100 mg/L IBP and 0.1% n-hexadecane (II). The scale bars on the CLSM images correspond to 5 μm.

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Fig 7 Expand

Table 7.

Morphometric parameters of R. cerastii IEGM 1278 cells grown in the RS medium supplemented with IBP and n-hexadecane.

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Table 7 Expand

Fig 8.

Correlation of membrane permeability with zeta potential of R. cerastii IEGM 1278.

Cells were grown in the RS medium supplemented with 0.1% n-hexadecane (A) and 100 mg/L IBP and 0.1% n-hexadecane (B).

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Fig 8 Expand