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Table 1.

Formulation of ionic mother liquor.

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Table 2.

Properties of simulated fracturing fluid.

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Table 2 Expand

Fig 1.

FE-SEM images of the original fracturing fluid at (a, b) low and (c, d) high magnifications. EDX Mapping results of the original fracturing fluid: (e) Mapping of all elements, (f) Mapping of Cl, O, Na and Ca.

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Fig 2.

(a) FTIR spectra of the original fracturing fluid and pure HPG. (b) Schematic of broken keys for HPG.

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Fig 3.

XPS full-scan spectrum of (a) simulated fracturing fluid-0 and (d) simulated fracturing fluid (after gel-breaking). High-solution C 1s XPS spectra of (b) simulated fracturing fluid-0 and (e) simulated fracturing fluid. High-solution N 1s XPS spectra of (c) simulated fracturing fluid-0 and (f) simulated fracturing fluid.

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Fig 3 Expand

Fig 4.

Molecular weight (MW) distributions of organic matter in the (a) pure HPG (b) simulated fracturing fluid-0 and (c) simulated fracturing fluid. Five MW fractions (<1 kDa, 1–10 kDa, 10–100 kDa, 100–1000 kDa, and>1000 kDa) were identified in the pure HPG, simulated fracturing fluid-0 and simulated fracturing fluid.

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Fig 4 Expand

Table 3.

The parameter values of HPG E-DLVO model.

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Table 3 Expand

Fig 5.

Interaction energy curves between HPG colloidal particles.

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Fig 5 Expand

Fig 6.

(a) The flocculation efficiency, (b) TOC content and removal efficiency of different flocculants after treating simulated fracturing fluid.

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Fig 6 Expand