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Fig 1.

A. Metformin and B. metformin-D6 fragmentation ion scans. Y-axis is Relative intensity (cps); X-axis is mass-to-charge (m/z). Red arrow indicates peak for m/z 60.2, pink arrow indicates peak for m/z 71.2.

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Fig 1 Expand

Fig 2.

Variation of Metformin chromatography by A. Metformin tautomerization in terms of proton movement; B. Representative Chromatographs before and after optimization from left to right: plasma, brain, muscle, liver, and kidney. For each graph, Y-axis: Intensity abundance (cps) and X-axis: acquisition time (min).

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Fig 2 Expand

Fig 3.

Representative MRM LC-MS/MS overlaid chromatogram of metformin at a lower limit of quantitation concentration and representative individual matrix blank injection after ULOQ.

Each individual tissue was represented by colors- green-plasma; blue-brain; dark green-muscle; brown-liver; red-kidney; black-mobile phase A. Y-axis: Intensity abundance (cps) and X-axis: acquisition time (min).

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Fig 3 Expand

Table 1.

Intra-day and inter-day precision and accuracy of the method in plasma and tissue homogenate spiked with metformin.

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Table 1 Expand

Table 2.

Matrix effect (% MF) and recovery (%) of QC samples (n = 6) for metformin in spiked mouse plasma.

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Table 2 Expand

Table 3.

Metformin concentrations in plasma, brain, liver, kidney, and muscle after 7 or 30 days of metformin treatment in male and female mice.

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Table 3 Expand

Fig 4.

Linear regression of metformin levels between plasma and different organs (n = 24).

Plasma and A. brain, B. liver, C. kidney, and D. muscle. Y-axis units are ng/g, and X-axis units are ng/ml.

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Fig 4 Expand

Table 4.

Comparison of metformin assessment methods using LC-MS/MS.

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Table 4 Expand