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Fig 1.

Chemical structures of HEMA and crosslinkers EGDMA, VM, AM, and AHPM.

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Table 1.

All hydrogels were synthesized with a 12.5/4.2/26.3 molar ratio of HEMA/crosslinker/UPW, while the chemical crosslinker or ratio of crosslinkers was varied.

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Fig 2.

Young’s modulus vs. toughness under physiological conditions for HEMA-based hydrogels photocrosslinked at multiple time points.

Chemical formulations are outlined in Table 1. UV exposure times varied across different formulations to achieve the widest possible range in modulus; exposure times for each data point are presented in S1 Fig.

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Fig 3.

Toughness as a function of equilibrium water content for the hydrogels with formulations described in Table 1.

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Fig 4.

Human dermal fibroblast viability after 72 hours of co-culture with VM crosslinked and EGDMA/VM co-crosslinked HEMA hydrogels at low and high crosslinking densities.

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