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Fig 1.

Map of study area showing ecoregions and sampling sites.

Red circles: sites with Fediss, a440 and DOC data; black circles: additional sites with only a440 and DOC data.

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Table 1.

Summary statistics for a440, DOC, and Fediss and two basic limnological variables in the NLF and NCHF ecoregions.

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Fig 2.

Plot of eigenvalues for the first two principal components of a principal components analysis of five variables (a440, DOC, Fediss, chl-a, and SD) for the whole data set.

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Fig 3.

(a) a440 and (b) DOC vs. Fediss for sampling years 2104–2016; triangles = 2014, squares = 2015, circles = 2016; dashed lines are regression fits for all years (see Table 1 for regression statistics).

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Table 2.

Dissolved Fe-CDOM and Fe-DOC relationships.

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Table 2 Expand

Table 3.

Simple and multiple regression relationships for a440 vs. DOC and Fediss.

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Table 3 Expand

Fig 4.

(a) a440/DOC vs. Fediss for all data, R2 = 0.64; (b) a440/DOC vs. Fediss for sites with a440 > 3.0 m-1, R2 = 0.46. (R2 are for fit of a440/DOC to ln(Fediss)).

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Fig 5.

(a) SUVA254,DOM vs. Fediss for sites with a440 > 3.0 m-1, R2 = 0.45 (R2 is for fit to ln(Fediss)); (b) fraction of SUVA254 for all sites caused by DOM (i.e., corrected for FeIII contribution) vs. Fediss.

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Fig 6.

a440 vs. Fediss for six waters in iron addition experiment; slopes and statistical information on best-fit lines in Table 4.

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Table 4.

Chemical characteristics of lakes and results for iron addition experiment.

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Table 4 Expand

Fig 7.

Fediss vs. a440 for 2015 data; best-fit regression line and statistics given in Table 2.

Circled data: outliers examined for effects of Fediss on a440 (S6 Table). Dotted line: best-fit linear relationship: Fediss = 36.8a440−30.7; R2 = 0.79. Dashed lines illustrate change in a440 for some outliers when Fediss was changed to “best-fit” value.

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