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Table 1.

Aroma compounds identified in clove essential oil and relative %.

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Table 1 Expand

Table 2.

Aroma compounds identified in spearmint essential oil and relative %.

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Table 2 Expand

Fig 1.

Major compounds of clove EO (A) and spearmint EO (B) with wave number regions for the CLS univariate and multivariate methods. Unloaded matrix represented with a dashed line.

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Fig 1 Expand

Table 3.

Main IR absorption bands used as reference for the elaboration of the ATR-FTIR method.

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Table 3 Expand

Fig 2.

Evolution of the normalization spectral band (2900–2950 cm-1).

Solid line represents the matrix after the elaboration process (n = 15) and the dotted line the matrix after three months (n = 15).

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Fig 2 Expand

Fig 3.

Results of the calibration and cross-validation CLS quantification method and GC-FID reference method.

Clove EO (A) and spearmint EO (B). ATR-FTIR calibration values (●), ATR-FTIR validation values (○), and GC-FID quantification values (Δ).

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Fig 3 Expand

Table 4.

Statistical data of ATR-FTIR CLS model for encapsulated clove and spearmint EOs.

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Table 4 Expand

Fig 4.

Clove EO release determined by ATR-FTIR (●) and GC-FID methods (○ = all components quantified, ♦ = eugenol, eugenol acetate, and methyl 2-hydroxybenzoate quantified).

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Fig 4 Expand

Fig 5.

Correlation of release through time of clove EO by the equation of Avrami.

ATR-FTIR quantification method values (●; dashed point line), GC-FID all components quantified (○; straight line), GC-FID eugenol, eugenol acetate, and methyl 2-hydroxybenzoate quantified (▲; dashed line).

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Fig 5 Expand

Table 5.

Statistical data of clove essential oil release experiment by ATR-FTIR and GC-FID method.

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Table 5 Expand