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Fig 1.

Raman spectroscopy.

A comparison of the Raman spectra of (a) GO with cGO crosslinked with Ca at 24, 34 and 55°C, and (b) GO with cGO crosslinked with Ca, Zn and Sr at 24°C.

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Fig 1 Expand

Fig 2.

EDS analysis.

Results in wt.% for GO and cGO crosslinked with Ca2+, Zn2+ and Sr2+.

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Fig 2 Expand

Fig 3.

Field emission scanning electron microscopy.

Images at a magnification of 50000 of (a) GO and cGO crosslinked with (b) Ca2+, (c) Zn2+ and (d) Sr2+ synthesised at 24°C.

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Fig 3 Expand

Fig 4.

High-resolution transmission electron microscopy.

Micrographs at two magnifications (a&b) with STEM dark field (c) of GO crosslinked with Zn2+ and uncrosslinked GO nanosheets (d).

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Fig 4 Expand

Fig 5.

Morphology and differential scanning calorimetry.

Confocal microscopy of (a) GO/Alg, (b&d) cGO/Alg, (c) DSC thermograms on heating of these samples at 10°C/min and (e) their morphology after swelling in water for 3 hours.

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Fig 5 Expand

Fig 6.

Dynamic mechanical analysis.

Temperature dependence of the storage modulus (solid symbols) and the loss tangent (open symbols) of cGO/Alg (◯) and GO/Alg (◇). Only one point out of ten is plotted to obtain a clearer representation.

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Fig 6 Expand

Fig 7.

Fourier transform infrared spectroscopy.

Spectra of cGO/Alg and GO/Alg from 650 to 4000 cm-1.

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Fig 7 Expand