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Fig 1.

The schematic structure of human insulin.

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Fig 2.

The construction scheme for the expression plasmid pIBAINS.

The resulting expression plasmid pIBAINS contains a hybrid protein SOD::INS gene under the control of the deoP1P2 promoter. Abbreviations used: AmpR, ampicillin resistant; TetR, tetracycline resistant; trpA—transcription terminator trpA; SOD, superoxide dismutase gene; A chain, B chain—chains of human insulin gene; ORI, replication origin.

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Table 1.

Nucleotide sequences of primers used for the point mutagenesis reaction.

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Table 1 Expand

Table 2.

Changes in amino acid sequence in new insulin analogs in reference to human insulin.

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Table 2 Expand

Fig 3.

a-d. Glycemia profiles after single dose administration of tested insulin analogs (GKR, GEKR, SR and AKR), positive (insulin glargine or insulin detemir) and negative (0.9% NaCl) control in streptozotocin-induced diabetic rats. Mean glycemia (± SEM). Star–statistical significance (p<0.05) confirmed in a Newman-Keuls test between one of the tested groups (GKR, GEKR, SR or AKR) and a negative control group (0.9% NaCl) at the individual sampling time point. Diamond–statistical significance (p<0.05) confirmed in a Newman-Keuls test between one of the tested groups (GKR, GEKR, SR or AKR) and a positive control group (insulin glargine or detemir) at the individual sampling time point. N–Number of tested animals per group.

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Fig 4.

a-d. The influence of multiple dose administration of tested insulin analogs (GKR, GEKR, SR and AKR) positive (insulin glargine or insulin detemir) and negative (0.9% NaCl) controls on glucose concentration in streptozotocin-induced diabetic rats, together with the period after termination of analogs administration. Mean glycemia (± SEM). Star–statistical significance (p<0.05) confirmed in a Newman-Keuls between one of the tested groups (GKR, GEKR, SR or AKR) and a negative control group (0.9% NaCl) at the individual sampling time point. Diamond–statistical significance (p<0.05), confirmed in a Newman-Keuls test during the administration period or in a t-test after stopping insulin administration, between one of the tested groups (GKR, GEKR, SR or AKR) and a positive control (insulin glargine or detemir) at the individual sampling time point. N–Number of tested animals per group.

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Fig 5.

The scheme for development and production of new analogs.

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Table 3.

Physicochemical properties of insulin analogs.

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Table 3 Expand

Table 4.

Chemical stability of drug product of insulin analogs during storage at 37°C: Formation of related proteins (content of related proteins in total including desamido A21).

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Table 4 Expand

Table 5.

Chemical stability of drug product of insulin analogs during storage at 37°C: Formation of covalent dimers and polymers (content of covalent dimers and polymers in total).

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Table 5 Expand