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Fig 1.

Schematic illustration of the hierarchical structure of a tree and the interaction between cellulose nanofibers and cement particles.

(a) The hierarchical structure of celluloses. (b) A network of cellulose nanofibers and cement formed with carboxyl groups and cement hydrates.

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Fig 1 Expand

Fig 2.

The morphology of cellulose nanofibers and the effect of CNFs on early hydration of cement particles.

(a) Size distribution of CNFs; (b) TEM image of CNFs; (c) Heat flow curves of CNF-cement pastes for the first 72 hrs’ hydration; (d) Scheme of CNFs promoting the setting of the cement paste by coordination with Ca2+.

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Fig 2 Expand

Table 1.

Water consistency and initial and final setting times for cement pastes.

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Table 1 Expand

Fig 3.

The flexural (a) and compressive (b) strengths of cement pastes with different CNF fractions addition at aging times of 3, 7, and 28 days.

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Fig 3 Expand

Fig 4.

DTA-TGA results of cement pastes with different CNF weight fractions from 100 to 800°C.

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Table 2.

WCH and Wb contained per gram cement paste with different CNF weight fractions.

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Table 2 Expand

Table 3.

Degree of hydration of cement pastes at different aging times.

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Table 3 Expand

Fig 5.

The microstructure of cement pastes after aging 28 days.

(a) SEM image of the cement paste. (b) SEM image of cement paste with 0.15% of CNFs; (c) and (d) Pore diameter distributions of cement pastes with different CNF content.

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Fig 5 Expand

Table 4.

The effect of CNFs addition on the pore structure.

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Table 4 Expand

Fig 6.

The relationship between mechanical strength (flexural strength and compressive strength) and DOH.

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Fig 6 Expand