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Fig 1.

Droplet size distributions of emulsions prepared with 7% (w/w) oil content at different OSA-modified starch concentrations.

A) Emulsions stabilized with granules. B) Emulsions stabilized with starch on the dissolved state. C) Mean volume diameter, D[4,3], of emulsions prepared with 7% (w/w) oil content at different OSA-modified starch concentrations stabilized both with granules or starch dissolved. D[4,3], was measured just after preparation and after 1 month under storage (1M).

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Fig 1 Expand

Fig 2.

Micrographs of emulsions stabilized with OSA-modified starch granules (A-C) and OSA-modified starch in the dissolved state (B-D).

A,B) Emulsions prepared at 7% (w/w) oil and stabilized using 50 mg starch/ml oil. C,D) Emulsions prepared at 33% (w/w) oil and stabilized with 100 mg starch/ml oil. Scale bar: 10 μm.

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Fig 2 Expand

Fig 3.

Kinetic ΔBS profiles of a 7% (w/w) oil emulsions.

A) Emulsions stabilized with OSA-modified starch granules at a concentration of 50 mg /ml oil. B) Emulsions stabilized with OSA-modified starch on the dissolved state at a concentration of 200 mg /ml oil. C, D) Turbiscan glass cells showing these emulsions respectively aspect after the monitoring time (1h). Note: Oil red EGN was added to visualize the eventual presence of free oil.

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Fig 3 Expand

Table 1.

Backscattering variations, ΔBS, changes in diameters, Δd/do, and migration velocities in the middle of the cell for emulsions formulated with 7–33% (w/w) oil content at different concentrations of OSA-modified and native starch dissolved (molecules).

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Table 1 Expand

Fig 4.

Droplet size distributions of emulsions with 33% (w/w) oil content prepared at different OSA-modified starch concentrations.

A) Emulsions stabilized using granules. B) Emulsions stabilized using starch in solution. Droplet size distributions were measured after preparation and after 1 month under storage (1M).

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Fig 4 Expand

Fig 5.

Kinetic ΔBS profiles of emulsions with 33% (w/w) oil content at different OSA-modified starch granules concentrations along the height of the cell.

A) Emulsions prepared at concentration of 100 mg starch/ml oil. B) Emulsions prepared at a concentration of 400 mg starch/ml oil. C) Turbiscan glass cells showing the emulsions aspect after the monitoring time. Note: Oil red EGN was added to visualize the eventual presence of free oil.

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Fig 5 Expand

Fig 6.

Kinetic ΔBS profiles of 33% (w/w) oil emulsions prepared at different OSA-modified starch concentrations on the dissolved state along the whole height of the cell.

A) Emulsions stabilized using 50 mg starch/ml oil. B) Emulsions stabilized using 100 mg starch/ml oil. C) Turbiscan glass cells showing the emulsions aspect after the monitoring time. Note: Oil red EGN was added to visualize the eventual presence of free oil.

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Fig 6 Expand

Fig 7.

Mean volume diameter, D[4,3], of emulsions prepared with 7% (w/w) oil content at different OSA-modified and native starch concentrations.

A) Emulsions stabilized with both types of starches in granules and on the dissolved state. B) Emulsions stabilized with mixtures of both; G:granules; D:dissolved.

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Fig 7 Expand

Fig 8.

Micrographs of emulsions stabilized by mixtures of OSA-modified starch in the form of granules and on the dissolved state adding both at the same time at different concentrations.

A) 50 mg starch/ml oil. B) 100 mg starch/ml oil. C) 200 mg starch/ml oil. D) 400 mg starch/ ml oil. E) Adding first granules and then starch dissolved at 200 mg starch/ ml oil. Scale bar = 10 μm.

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Fig 8 Expand