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Table 1.

Different media used for the optimization of fungal VCR and VBL production.

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Fig 1.

Isolation of endophytic fungi from C. roseus plant.

Arrowheads indicate the emergence of endophytic fungi from the plant cuttings. A-leaf, B-stem, C-pedicel and D-flower petal.

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Fig 2.

PCR products of approximately 550 to 600 bp of ITS region in endophytic fungi of C. roseus.

Lane M: 100-bp DNA marker. Lanes 1 to 22: PCR products of CrP1 to CrP22.

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Table 2.

Details of the endophytic fungi isolated from C. roseus and the antiproliferative effects (IC50 values) of their crude extracts against human HeLa cells.

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Table 2 Expand

Fig 3.

Effects of the ethyl acetate extracts of mycelium on the antiproliferative activity of HeLa cells.

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Fig 4.

Effects of the ethyl acetate extracts of filtrate on the antiproliferative activity of HeLa cells.

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Fig 5.

Genomic PCR analyses to determine the presence of the TDC gene.

Lane M: 100-bp ladder; Lanes 1–22: the PCR amplification products of the TDC gene in 22 endophytic fungal isolates. Arrowheads show the amplified products in T. radicus—CrP20 and C. roseus (which served as the positive control).

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Fig 6.

Macromorphology of Ten-day-old TIA-producing fungus T. radicus—CrP20 on PDA medium, showing mycelial growth and green-colored spores.

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Fig 7.

Micromorphology of T. radicus—CrP20, showing phialides with chains of conidia under light microscope (40X magnification).

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Fig 8.

Thin-layer chromatography analysis of T. radicus—CrP20 crude extract on a silica gel aluminum sheet.

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Fig 9.

LC-ESI-MS analysis. of fungal VCR.

The mass spectrum of the fungal extract showed a (M+H+) peak at a molecular mass of 825.46, which was identical to that observed in the mass spectrum of the VCR standard.

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Fig 10.

LC-ESI-MS analysis of fungal VBL.

The mass spectrum of the fungal extract showed a (M+H+) peak at a molecular mass of 811.51, which was identical to that observed in the mass spectrum of the VBL standard.

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Fig 11.

HPLC profile of T. radicus—CrP20 culture extract showing VCR (RT-11.43) and VBL (RT-12.83).

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Fig 12.

Production of VBL and VCR by T. radicus—CrP20 grown in different media.

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Fig 13.

Cytotoxic activity of ‘fungal VCR’ in different cancer cell lines.

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Fig 14.

Cell cycle distribution of HeLa cells treated with different concentrations of ‘fungal VCR’.

The sub-G0/G1, G1, S and G2/M phases are represented on the histogram as P5, P2, P4 and P3, respectively. A—control, B—fungal VCR (5 μg/ml), C—fungal VCR (10 μg/ml), D—fungal VCR (25 μg/ml) and E—percent apoptosis.

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Fig 15.

Induction of apoptosis in HeLa cells treated with different concentrations of ‘fungal VCR’, as determined by annexin V-FITC/PI dual staining.

A- untreated cells, B—cells + FITC, C—cells + PI, D—cells + FITC + PI, E—cells + FITC + PI + fungal VCR (5 μg/ml), F—cells + FITC + PI + fungal VCR (10 μg/ml), G—cells + FITC + PI + fungal VCR (25 μg/ml) and H—percentage of cells undergoing early apoptosis.

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Fig 16.

Induction of mitochondrial membrane depolarization in HeLa cells treated with various concentrations of ‘fungal VCR’.

A—cells alone, B—cells + JC1 stain, C—cells + JC1 + 25 μM valinomycin (+ ve control), D—cells + JC1 + fungal VCR (5 μg/ml), E—cells + JC1 + fungal VCR (10 μg/ml), F—cells + JC1 + fungal VCR (25 μg/ml), G—standard VCR (2 nM) and H—percent loss of mitochondrial membrane depolarization.

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Fig 17.

DNA fragmentation in HeLa cells treated with ‘fungal VCR’.

A—control, B—cells treated with fungal VCR (10 μg/ml), C—cells treated with fungal VCR (25 μg/ml) and D—1-kb DNA ladder.

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