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Fig 1.

Chemical Structure of Acid Blue 113.

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Table 1.

EDX analysis of ZSM-5 and Fe-ZSM-5.

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Table 1 Expand

Table 2.

Pore structure characteristics of the ZSM-5 support and Fe-ZSM-5 catalyst.

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Table 2 Expand

Table 3.

Taguchi Design Factors and their levels.

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Table 4.

L27 orthogonal design, experimental results, and Taguchi analysis for run 1 to 16,

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Table 4 Expand

Table 5.

L27 orthogonal design, experimental results, and Taguchi analysis for run 17 to 27.

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Table 5 Expand

Table 6.

Theoretical framework of the Taguchi method coupled with principle component analysis (PCA).

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Table 6 Expand

Fig 2.

SEM images of (a) the Fe(byp) complex, (b) ZSM-5, and (c) Fe-ZSM-5.

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Fig 2 Expand

Fig 3.

FTIR data for (a) the ZSM-5, (b) Fe-ZSM-5, and (c) Fe(byp) complex.

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Fig 3 Expand

Table 7.

The obtained S/N ratios, normalized S/N ratios, and TPCI values for run 1 to 15.

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Table 7 Expand

Table 8.

The obtained S/N ratios, normalized S/N ratios, and TPCI values for run 16 to 27.

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Table 8 Expand

Table 9.

Eigenvalues and Eigenvectors obtained through PCA processing of the normalized S/N ratios.

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Table 9 Expand

Fig 4.

Mean TPCI plots with respect to parameter changes.

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Fig 4 Expand

Table 10.

List of TPCI responses.

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Table 10 Expand

Table 11.

Optimized values for heterogeneous Fenton oxidation.

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Table 11 Expand

Table 12.

ANOVA analysis.

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Table 12 Expand

Fig 5.

Interaction of parameters with respect to TOC.

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Fig 5 Expand

Fig 6.

Interaction of parameters with respect to decolorization.

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Fig 7.

Interaction of parameters with respect to degradation.

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Fig 8.

SEM images of the (a) fresh and (b) spent Fe-ZSM-5.

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Fig 9.

FTIR spectra of the (a) fresh and (b) spent Fe-ZSM-5.

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Table 13.

Comparison of synthesized Fe-ZSM-5 with other catalysts used for the degradation of Acid Blue 113.

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Table 14.

Efficiency comparison chart of different Fe-ZSM-5 catalysts used for the degradation of dyes.

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Table 14 Expand

Fig 10.

Degradation and TOC removal of mixture of dyes using Fe-ZSM-5.

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Fig 10 Expand