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Table 1.

Composition of normal and high phosphate-modified AIN-93G rodent diets.

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Table 2.

ICP-MS and ICP-OES operational conditions.

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Fig 1.

Tumor incidence in the lungs of K-rasLA1 mice provided with an ND or HPD.

Mice (n = 6 per group) were fed an ND (0.3% Pi) or HPD (1% Pi) for 1, 2, or 4 months. (A) Adenocarcinoma and adenoma in the lung tissue. (B) Total number of tumors, number of tumors with diameter >1.5 mm, and tumor volume in ND- and HPD-fed mice. The results are mean ± standard deviation (SD) of six independent measurements. Error bar represent SD. *p < 0.05; **p < 0.01; ***p < 0.001. (C) Tumors on the lungs of ND- and HPD-fed mice, as visualized by H&E staining. Scale bar: 100 μm.

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Table 3.

Daily food and inorganic phosphate intake and body weight in K-rasLA1 mice fed a normal or high-phosphate diet for 1, 2, or 4 months.

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Table 4.

Tumor incidence in the lungs of K-rasLA1 mice fed a normal or high-phosphate diet for 1, 2, or 4 months.

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Fig 2.

Changes in ion levels in the liver and lungs of K-rasLA1 mice provided with an ND or HPD for 4 months.

LA-ICP-MS analyses represent mean values from three trials of solution ICP-MS/ICP-OES data (n = 6 per group). The vertical bar in graded color from blue to red represents the ion level from low to high, respectively.

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Table 5.

Changes in ion levels in the livers and lungs of K-rasLA1 mice fed a normal or high-phosphate diet for 1, 2, or 4 months

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Fig 3.

Western blot analysis of cellular metabolism-related proteins.

Protein expression of p-acetyl CoA, acetyl CoA, SDHA (complex II), cytochrome c (complex III), COX IV (complex IV), and Rieske (Fe-S complex) relative to glyceraldehyde-3-phosphate dehydrogenase (GAPDH) in liver tissue homogenates of K-rasLA1 mice fed an ND or HPD for 1, 2, or 4 months (n = 6 per group), as determined by western blotting and quantified by densitometry. The results are mean ± SD. Error bar represent SD. *p < 0.05; **p < 0.01.

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Fig 4.

Western blot analysis of EMT- and autophagy-related proteins and qRT-PCR analysis of epithelial marker.

(A) Protein expression of the autophagy markers LC3 and ATG5 in lung tissue homogenates as determined by western blotting, using actin as a loading control. (B) LC3 expression (green) in lung tissue sections was assessed by immunocytochemistry. The highest immunoreactivity was observed in the 4-month HPD group relative to the corresponding control (ND) group. Scale bar: 10 μm. (C) Protein expression of the EMT marker N-cadherin in lung tissue homogenates of K-rasLA1 mice fed an ND or HPD for 1, 2, or 4 months (n = 6 per group), as determined by western blotting, using actin as a loading control. The results are mean ± standard deviation SD. Error bar represent SD. *p < 0.05; **p < 0.01; ***p < 0.001. (D) qRT-PCR analysis of epithelial markers, E-Cadherin. The results are mean ± standard deviation SD. Error bar represent SD. *p < 0.05; ***p < 0.001.

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Fig 5.

Analysis of protein translation in the lungs of K-rasLA1 mice provided with an ND or HPD.

The expression of the translation-related proteins p70S6K, eIF4E, p-4E-BP-1/2, and 4E-BP-1/2 in lung tissue homogenates of K-rasLA1 mice fed an ND or HPD for 1, 2, or 4 months was determined by western blotting and quantified by densitometry (n = 6 per group) relative to the expression level of actin. The results are mean ± standard deviation SD. Error bar represent SD. *p < 0.05; **p < 0.01; ***p < 0.001.

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Fig 6.

Analysis of proliferation and angiogenesis.

Proliferation and angiogenesis were evaluated in the lungs of K-rasLA1 mice fed an ND or HPD for 1, 2, or 4 months (n = 6 per group). (A) Expression of proteins associated with proliferation (PCNA) and angiogenesis (FGF-2) in lung tissue homogenates was evaluated by western blotting, using actin as a loading control. (B) PCNA-expressing cells in the tumor region (upper right corner of each panel) were visualized by immunohistochemistry. Scale bar: 20 μm. The results are mean ± standard deviation SD. Error bar represent SD. *p < 0.05; **p < 0.01.

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Fig 7.

Apoptosis in the lungs of K-rasLA1 mice provided with an ND or HPD.

Apoptosis in the lungs was analyzed in K-rasLA1 mice fed an ND or HPD for 1, 2, or 4 months (n = 6 per group). (A) The expression of the mitochondrial apoptosis-related proteins Bad, Bax, and cytochrome c was evaluated by western blotting of lung tissue homogenates, with actin used as a loading control. (B) Immunohistochemical analysis of caspase-3 expression in the tumor region. Scale bar: 20 μm. The results are mean ± standard deviation SD. Error bar represent SD. *p < 0.05; **p < 0.01.

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