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Fig 1.

Synthesis of BC-EDTA.

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Fig 2.

Ultraviolet-Visible (UV) Absorption Spectrum of BC-EDTA.

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Fig 3.

Outline of labeling bare particles with BC-EDTA.

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Fig 4.

Scheme of labeling of antibody with BC-EDTA/Eu3+-nanosphere.

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Fig 5.

Schematic representation of the immunoassay system for HBsAg by BC-EDTA/Eu3+-nanosphere.

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Fig 6.

TEM of bare silica nanosphere.

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Fig 7.

Relationship between fluorescence intensity of nanosphere and coating times.

BC-EDTA/Eu3+-nanosphere was diluted in 0.05 mol/L carbonate buffer, pH9.5, with the concentration of 0.01%.

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Fig 8.

TEM of BC-EDTA/Eu3+-nanosphere.

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Fig 9.

Excitation and Emission spectra of BC-EDTA/Eu3+ (A) and BC-EDTA/Eu3+-nanosphere (B).

(A) The concentration of BC-EDTA/Eu3+ is 10-3mol/L. The buffer was 0.05 mol/L carbonate buffer, pH9.5. (B) The concentration of BC-EDTA/Eu3+-nanosphere is 0.005%. The buffer was 0.05 mol/L carbonate buffer, pH9.5.

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Table 1.

Unspecific conjugation of antibody labeled BC-EDTA/Eu3+-nanosphere, unlabeled BC-EDTA/Eu3+-nanosphere to antibody coated microwell plate.

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Table 2.

Specific conjugation of antibody labeled BC-EDTA/Eu3+-nanosphere to HBsAg coated mircowell plate.

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Table 3.

Functional sensitivity of BC-EDTA/Eu3+-nanosphere.

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Table 4.

Analytical precision of determination of HBsAg in human serum (n = 20).

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Table 5.

Analytical recovery rate of determination of HBsAg in human serum (n = 10).

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Fig 10.

Calibration curves for HBsAg.

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Fig 11.

Regression analysis result of BC-EDTA/Eu3+-nanosphere based TrFIA and DELFIA.

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