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Fig 1.

FESEM and HRTEM images of ZnO-based nanostructures.

FESEM images of (a) ZnO nanorods, (b) ZnO nanocons, (c) ZnO–ZnS core–shell nanocones, and (d) HRTEM image of the ZnO-ZnS core-shell structure.

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Fig 1 Expand

Fig 2.

XRD patterns of the ZnO–ZnS core-shell nanocone arrays on FTO substrate.

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Fig 2 Expand

Fig 3.

Room-temperature PL spectra of the bare ZnO and the shelled ZnO nanocones.

The inset shows the relative PL intensity ratio between the peak intensity of UV and DLE.

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Fig 3 Expand

Fig 4.

The band-edge alignments at the heterointerface between ZnO and ZnS semiconductors.

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Fig 4 Expand

Fig 5.

Optical absorption and reflectance spectra of the samples.

(a) Absorption and (b) reflectance spectra of the ZnO nanorods, nanocons, and ZnO–ZnS core–shell nanocones.

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Fig 5 Expand

Fig 6.

The photocurrent density–voltage characteristics of the ZnO nanostructures

(a) Comparison of photocurrent density-voltage plot of the DSSCs based on ZnO nanorods, nanocons, and ZnO–ZnS nanocones (b) schematic diagram of the energy levels of the hetrostructure ZnO/ZnS photoelectrode in a DSSC.

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Fig 6 Expand

Table 1.

Performances of the DSSCs based on ZnO nanorods, nanocons, and heterostructure ZnO–ZnS nanocones.

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Table 1 Expand

Fig 7.

EIS Nyquist plots of DSSCs based on different ZnO nanostructures.

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Fig 7 Expand