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Figure 1.

General XPS spectra of (a) WMS, (b) SNCH2SO4,3, (c) SNCH2SO4,7, and (d) SNCHCl,7.

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Table 1.

Elemental surface composition (atomic %) and oxygen to carbon ratio of starch, HCl- and H2SO4-hydrolyzed SNC.

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Table 1 Expand

Figure 2.

The high-resolution C 1 s deconvoluted XPS spectra of (a) WMS, (b) SNCH2SO4,3, (c) SNCH2SO4,7, (d) SNCHCl,7.

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Figure 2 Expand

Table 2.

Surface functional group composition as obtained from the deconvolution of the C 1

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Table 2 Expand

Figure 3.

The high-resolution S 2p deconvoluted XPS spectra of (e) WMS, (f) SNCH2SO4,3, (g) SNCH2SO4,7, and (h) SNCHCl,7.

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Figure 3 Expand

Figure 4.

FT-IR spectra of (a) WMS, (b) SNCH2SO4,3, (c) SNCH2SO4,7, and (d) SNCHCl,7.

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Figure 5.

Formation of sulfate esters and adsorption of formic and levulinic acids on the surface of SNC (a: Formation of sulfate ester, b: adsorption of formic and levulinic acids).

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Figure 5 Expand

Figure 6.

Zeta potential of SNCH2SO4,7 (gray color) and SNCHCl,7 (white color) suspensions at pH 6.5 and 10.6 placed for 2 h and 48 h, respectively.

Data are represented as the mean ± standard deviation (n = 3).

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Figure 6 Expand

Figure 7.

TEM pictures and sedimentation properties of HCl (a and b) and H2SO4 (c and d) hydrolyzed SNC suspensions after 2 h and 48 h.

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Figure 7 Expand