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Table 1.

Custom designed protein arrays kit, which consist of 20 different cytokines/factors.

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Figure 1.

Inhibitory effect of melatonin on viability of the MDA-MB-231 cell line.

The MDA-MB-231 cells were treated with five concentrations of melatonin for 24 h and cell viability was measured by MTT assay. Data are shown as mean ± S.D. *p<0.05, 1 mM of melatonin vs. Control; #p<0.05, 1 mM of melatonin vs other melatonin's concentrations.

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Figure 2.

Antitumor effects of melatonin on mammary tumor growth.

Melatonin reduced the tumor growth in breast cancer nude mice. Each point in the curves represents the mean ± SD (control n = 8; melatonin n = 5). The melatonin inhibited tumor growth, *p<0.05 vs Control. # Significant increase in tumor volume on control group at 14 and 21 after tumor implantation and initiation of treatment with vehicle (p<0.05). Detail: Representative samples of mammary tumors developed by MDA-MB-231 cells implantation on the right flank of mice. A, B. Melatonin treated mammary tumors, B. Mammary tumor which regressed with melatonin treatment. C, D. Vehicle treated mammary tumors.

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Figure 3.

SPECT analysis of in vivo accumulation of Tc-99m-HYNIC-VEGF-c.

VEGF-c (which targets both VEGFR2 and VEGFR3) was tagged with HYNIC chelators and then labeled with Tc-99m and injected intravenously in melatonin and vehicle treated mice. One hour after injection, SPECT images were obtained using dedicated animal scanner. Vehicle treated mice showed increased accumulation of Tc-99m-HYNIC-VEGF-c in the mammary tumor (A, Intersection of lines indicate the tumor, with a volume of 865.69 mm3 at the 21th day) compared to that of melatonin treated mammary tumors (B, Intersection of lines indicate the tumor, with a volume of 130.69 mm3 at the 21th day) C. Semi-quantitative analysis of total radioactivity normalized to contralateral muscles showing the intensity of radioactivity in the vehicle and melatonin treated animals.

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Figure 4.

Comparison between proteins expression in mammary tumor in animals treated with melatonin or vehicle.

White column = vehicle treatment; Black column = melatonin treatment. Data are shown as mean ± S.D. *p<0.05, vs. Control.

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Figure 5.

Immunohistochemistry staining with VEGFR2 (arrows) in vehicle treated and melatonin treated tumors.

Images were taken with 40× magnification. A significant decrease was observed at the tumor in melatonin treated tumors compared to vehicle treated tumors (*p<0.05). Error bars: ± standard error.

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Figure 6.

Immunohistochemistry staining with VEGFR3 (arrows) in vehicle treated and melatonin treated tumors.

Images were taken with 40× magnification. Melatonin do not decreased significantly the expression of VEGFR3 (p>0.05). Error bars: ± standard error.

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Figure 7.

Immunohistochemistry staining with vWF in vehicle treated and melatonin treated tumors.

Images were taken with 40× magnification. Quantitative estimation of micro-vessel density (MVD) by counting positive vessels (arrows) revealed a decrease in MVD after melatonin treatment compared to the vehicle treated tumor (*p<0.05). Error bars: ± standard error.

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Figure 8.

Immunohistochemistry staining with Ki-67 in vehicle treated and melatonin treated tumors.

Images were taken with 40× magnification. There was a decreased cell proliferation in tumors treated with melatonin (*p<0.05). Error bars: ± standard error.

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