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Figure 1.

Participation of MEP-dependent isoprene biosynthesis pathway into two modules.

Gene symbols and the enzymes they encode (all genes were from E. coli except where noted): dxs, DXP synthase; ispC, DXP reductionisomerase; ispD, DXP-ME synthase; ispE, CDP-ME kinase; ispF, MECPP synthase; ispG, HMBPP synthase; ispH, HMBPP reductase; idi, IPP isomerase; ispS, isoprene synthase (P. alba). Pathway intermediates: G3P, glyceraldehyde-3-phosphate; DXP, 1-deoxy-D-xylulose 5-phosphate; MEP, 2-C-methyl-D-erythritol 4-phosphate; CDP-ME, 4-diphosphocytidyl-2-C-methyl-D-erythritol; CDP-MEP, 4-diphosphocytidyl-2-C-methyl-D-erythritol 2-phosphate; MECPP, 2-C-methyl-D-erythritol 2,4-cyclopyrophosphate; HMBPP, 1-hydroxy-2-methyl-2-(E)-butenyl 4-pyrophosphate; IPP, isopentenyl pyrophosphate; DMAPP, dimethylallyl pyrophosphate; DHAP, dihydroxyacetone 3-phosphate.

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Figure 1 Expand

Figure 2.

Four glycolytic pathways present in E. coli.

EMP, Embden-Meyerhof pathway; PPP, pentose phosphate pathway; EDP, Entner-Doudoroff pathway.

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Figure 2 Expand

Figure 3.

Isoprene titers and yields from different feeding modules.

Module 1, EMP of strain FMIS 1; Module 2, EDP+PPP of strain FMIS 2; Module 3, EDP of strain FMIS 3, these three strains used glucose as carbon source. Module 4, PPP of strain FMIS 4; Module 5, Dahms pathway of strain FMIS 5, these two strains used D-xylose as carbon source. All strains are listed in Table S1 in File S1. A 160 mL serum bottle containing 40 mL of semi-defined medium, consisted of M9 salts, 5 g L−1 yeast extract, 10 g L−1 required carbon source and 1 mM thiamine pyrophosphate (TPP), was used for the cultivation of the strains for isoprene production.

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Figure 3 Expand

Table 1.

Substrate consumption, isoprene and biomass productions from different feeding modulesa.

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Table 1 Expand

Figure 4.

Pyruvate and G3P generation, energy and reducing equivalents production of different glycolytic pathways.

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Figure 4 Expand