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Figure 1.

Fresh berry weight (g) and total anthocyanin content (absorbance at 530 nm per g of freeze dried material) of berries at developmental stages of EL 32, EL 35, EL 36 and EL 38.

Bars represent standard deviation.

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Figure 1 Expand

Figure 2.

Relative quantification of malic acid, tartaric acid, fructose and glucose based on ion peak response.

Malate and tartrate contents are higher at pre-véraison stages peaking at EL 32 whereas contents in fructose and glucose increase at post-véraison stages reaching maximal levels at EL 38.

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Table 1.

List of metabolites identified by GC-EI-TOF/MS and GC-EI-MS during ripening of the three varieties.

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Figure 3.

Score plot of ICA showing metabolic discrimination of developmental stages and cultivars.

A Polar metabolites B Volatiles.

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Figure 4.

Heat map showing metabolite levels analyzed during berry ripening.

Each square represents the average of the biological replicates.

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Table 2.

Selection of genes differentially expressed during ripening of the three grape varieties (considering a fold change ≥1.5 and FDR <0.05 or fold change ≤−.1.5 and FDR<0.05).

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Figure 5.

PCA plot showing transcriptional discrimination of developmental stages and cultivars.

The first (PC1) and the second (PC2) principal components are represented.

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Figure 6.

Functional categories distribution in the common gene set of the 2255 modulated probesets and in the entire GrapeGen Chip®.

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Figure 7.

Real time qPCR validation of the expression profiles of ten genes in the three varieties under analysis.

Data are reported as means ± SE of three technical and two-three biological replicates. Transcript levels were calculated using the standard curve method and normalized against grapevine actin gene (VVTU17999_s_at) used as reference control. Flavonol synthase (VVTU16103_at); Palmitoyl-monogalactosyldiacylglycerol delta-7 desaturase, chloroplast (VVTU3709_at); Succinate semialdehyde dehydrogenase (VVTU35625_s_at); Tocophenol cyclase (VVTU22626_s_at); L-Galactono-1,4-lactone dehydrogenase (VVTU8069_at); Limonoid UPD-glycosyltransferase (VVTU17111_s_at); Terpene synthase (VvTPS10); Terpene synthase (VvTPS34); Cytochrome 450 monooxygenase CYP89H3 (VVTU21329_at) and Caffeic acid O-methyltransferase (VVTU36927_x_at).

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Figure 8.

Phenylpropanoids-related transcripts and metabolites showing significant differences between véraison and ripening (EL 36 vs EL 35) in Touriga Nacional cultivar; pathways are represented in VitisNet networks [81] with the Cytoscape software.

Parallelograms represent non-redundant transcripts differentially expressed. Ovals and hexagons represent metabolites and enzymes, respectively. Pink lines show metabolic reactions and blue lines catalytic reactions; bold arrows highlight the reactions starting from phenylalanine leading to anthocyanidin biosynthesis. Green represents transcripts down-regulated or decrease in metabolites values, whereas purple represents transcripts up-regulated or increase in metabolites values.

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Figure 9.

Candidate molecular and metabolic markers of pre-ripe and ripe berries established in three Portuguese varieties.

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