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Figure 1.

Abbreviated decay scheme of 225Ac.

225Ac emits 4 α particles in the process of decaying to the long-lived 209Bi.

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Figure 2.

Schematic of gold coated lanthanide phosphate NP.

The α emitter is loaded in the {La0.5Gd0.5}PO4 core, the GdPO4 layer(s) increase retention of the decay chain daughters, and the Au shell facilitates attachment of targeting agents.

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Figure 3.

TEM image of {La0.5Gd0.5}PO4 core NPs.

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Figure 4.

TEM of a characteristic cluster of NPs.

EELS analysis indicates the presence of La, Gd, and Au in all particles in the cluster.

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Table 1.

Growth of NP diameter as a function of shell addition as measured by TEM.

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Table 2.

Dynamic light scattering of NPs in 18 MΩ water.

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Figure 5.

MAb 201b antibody conjugation to multi-layered NPs.

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Figure 6.

Biodistribution of NPs following tail vein injection in mice at 1 hour (n = 3).

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Figure 7.

SPECT/CT images 1 hour post-injection of 80 µCi of {La0.5Gd0.5}(225Ac)PO4@GdPO4@Au-mAb-201b.

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