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Figure 1.

Transmission electron microscopy image of NM-containing organelles.

Transmission electron microscopy image of a pigmented organelle from SN containing the NM pigment (white arrow) and lipid droplets (black arrow). The tissue was prepared as described in ref. 2 (scale bar 500 nm).

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Figure 1 Expand

Table 1.

Amino acid content (µg/mg of isolated pigment) ± standard error of the mean (sem).

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Table 1 Expand

Table 2.

Elemental composition and C/N ratio of NM of SN, CAL and other brain areas a.

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Table 2 Expand

Table 3.

Theoretical percentage a of the various components in SN-NM, other-NM, and CAL-NM.

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Table 3 Expand

Figure 2.

IR spectra of the three NM types.

Comparison of IR spectra of SN-NM, other-NM (from PAL) and CAL-NM. Typical absorptions are indicated by asterisks (1230, 1194, 1163 cm−1) and arrows (1774, 1015 cm−1), for assignments see text.

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Figure 2 Expand

Table 4.

Detailed assignment of the IR absorption bands of NM.

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Table 4 Expand

Figure 3.

1D- and 2D-NMR spectra of NM.

Representative NMR spectra of NM, those shown are for the NM isolated from CAB: (A) 1D proton, (B) COSY, (C) 1H-13C HSQC, (D) 1H-13C HMBC, (E) DOSY.

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Figure 3 Expand

Table 5.

Experimental 13C ppm values of NM pigments as determined by 2D 1H-13C HSQC, compared to known values of bovine liver dolichol [27].

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Table 6.

Summary of COSY, HSCQ and HMBC interactions a.

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Figure 4.

1D proton HR-MAS and solution NMR spectra of NM from PUT.

(A) HR-MAS water-presaturation pulse sequence with composite pulse; (B) solution spectrum with water suppression by gradient-tailored excitation. In the HR-MAS spectrum most major signals are shifted slightly upfield.

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Figure 4 Expand

Figure 5.

1D proton HR-MAS NMR spectra of NM from PUT.

(A) HR-MAS diffusion-edited spectrum; (B) unfiltered HR-MAS spectrum; (C) HR-MAS CPMG sequence; (D) solution CPMG sequence. The vertical grey box shows the presence of two different signals around 5.0 ppm.

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Figure 5 Expand

Figure 6.

Solid state 13C NMR spectra of NM from PUT.

(A) regions of interest in the zg spectrum; (B) high power decoupled spectrum. The intense signal at 110 ppm derives from the teflon insert, * indicates the spinning side band. The second (right hand) spinning side band (at ∼ 30 ppm) disappears beneath sample signals.

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Figure 6 Expand

Table 7.

Results from the 13C solid state NMR spectrum.

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Table 7 Expand