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Table 1.

Binding free energies (kcal/mol) between PBP2x protein and cefuroxime (CES) in the two complexes.

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Table 1 Expand

Figure 1.

Sequence alignment between PBP2x-R61 (R61), PBP2x-A7 (A7), and the template protein (PDB code 1QMF).

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Figure 1 Expand

Figure 2.

Ramachandran plot of modeled PBP2x-R61 and PBP2x-A7.

The most favored regions are red. Additionally allowed, generously allowed, and disallowed regions are indicated as yellow, light yellow, and white, respectively.

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Figure 2 Expand

Figure 3.

Comparison of PBP2x-R61 and PBP2x-A7.

(A) The superimposition of initial structures of the complex between PBP2x-R61 (white color) and PBP2x-A7 (cyan color) with the drug (green color). (B) The structure of the cefuroxime drug.

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Figure 3 Expand

Figure 4.

RMSD values for PBP2x-R61-CES and PBP2x-A7-CES relative to the starting structure during MD simulation.

(A) The whole backbone atoms. (B) The drug molecule.

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Figure 4 Expand

Figure 5.

Relative decomposed energies of the corresponding residues between PBP2x-R61-CES and PBP2x-A7-CES.

The ovals characterize the two active site areas and the blocks mark the three essential mutated residues.

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Figure 5 Expand

Table 2.

The list of the residues with absolute energy larger than 1.0 kcal/mol or the residues with the difference between the two complexes larger than 0.5 kcal/mol.

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Table 2 Expand

Figure 6.

The distance variation of the five hydrogen bonds during MD simulation.

(A) for PBP2x-R61-CES. (B) for PBP2x-A7-CES. Bond 1: Ser396 O - CES O7; Bond 2: Gly350 N - CES O3; Bond 3: Thr351 OG1 - CES N2; Bond 4:Thr351 OG1 - CES O5; and Bond 5: Thr351 N - CES O5.

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Figure 6 Expand

Figure 7.

LIGPLOT representation of cefuroxime (CES) binding to PBP2x-R61 and PBP2x-A7.

Ligand, protein, and hydrogen bonds are in thick blue, thick brown, and broken green lines, respectively. Residues involved in hydrophobic contact are associated with a curved comb. (A) Open form of cefuroxime (CES) bound to PBP2x-R61. (B) Open form of cefuroxime (CES) bound to PBP2x-A7.

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Figure 7 Expand

Table 3.

The property of the mutated residues in the binding site of the two complexes PBP2x-R61-CES and PBP2x-A7-CES.

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Table 3 Expand