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Figure 1.

Construction of the S2.2-spacer aptamer and PTX-Apt-NPs.

(A) Structure of MUC1 aptamer S2.2-spacer. The S2.2-spacer is made of the MUC1 aptamer S2.2 (as the targeting agent) and a designed sequence of single strand DNA (as the linking spacer). (B) Preparation procedure for PTX-Apt-NP using the emulsion/evaporation method.

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Figure 2.

FCM analysis of MCF-7 and HepG2 cells incubated with random DNA, MUC1 aptamer S2.2, or S2.2-spacer.

(A) Histograms of FCM analysis. FITC-labeled random DNA, S2.2, or S2.2-spacer was incubated separately with MCF-7 (left) and HepG2 (right) cells. (B) The mean fluorescent intensity of MCF-7 and HepG2 cells incubated with random DNA and different aptamers.

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Figure 3.

Analysis of aptamer conjugation to microparticles or nanoparticles.

The PLGA microparticles (MPs) or nanoparticles (NPs) reacted with aptamers in the absence (-EDC&NHS) or presence (+EDC&NHS) of the catalysts. (A) Histograms of FCM analysis of MP reacted with FITC-labeled aptamers in the absence (-EDC&NHS, left) or presence (+EDC&NHS, right) of the catalysts. Plain microparticles that had not reacted with aptamers were used as control. (B) UV absorption of DNA at 260 nm (n = 3) on the particles that underwent conjugation process with aptamers. The control group (NPs) indicates plain nanoparticles that have not reacted with DNA aptamers.

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Figure 4.

In vitro drug release profile of the PTX encapsulated Apt-NPs.

The experiment was conducted in phosphate buffer saline (PBS, pH 7.4) containing 0.5% (w/v) poloxamer using the membrane diffusion technique, (n = 3).

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Figure 5.

FCM analysis of cellular uptake of Apt-NPs and NPs by MCF-7 (left) and HepG2 cells (right).

The cells were incubated with FITC encapsulated Apt-NPs or NPs at 50 µg/ml for 2 hours before subject to analysis.

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Figure 6.

Confocal fluorescent scanning microscopy images detecting cellular uptake of Apt-NPs (top row) or NPs (bottom row) in MCF-7 cells.

Green fluorescent FITC was encapsulated in Apt-NPs and NPs. The nuclei were stained blue with DAPI. The right column showed the merged images of the FITC and the DAPI channels. MCF-7 cells were exposed to FITC-encapsulated Apt-NPs or NPs at 100 µg/ml for 2 hours.

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Figure 7.

Cytotoxicity assays of MCF-7 (Left) and HepG2 cells (Right) treated for 4 hours with plain nanoparticles (NP), free paclitaxel (PTX), PTX-loaded NPs (PTX-NP), PTX-loaded NPs conjugated to random DNA (PTX-R-NP), or PTX-loaded NPs conjugated to MUC1 aptamer (PTX-Apt-NP).

The cells were subsequently washed and incubated in culture media for a total of 48 hours, before cell viability in each group was assessed with a standard MTS assay (n = 6, mean ± SD).

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